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Abstract
We tested the suitability of the multiple interactive continua approach (MINC) to simulate reactive mass transport in a disturbed post-mining coal zone. To the authors’ knowledge, this approach has not been employed in such mining settings despite its relative success in other environmental fields. To this end, TOUGHREACT software was used to set up a MINC model of the unsaturated overburden of the Ibbenbüren Westfield. With it, we examined and evaluated water–rock interactions in both the fractured and porous continua as the main driver of elevated hydrogen, iron, sulfate, and chloride concentrations in the coal mine groundwater. Long and seasonal geochemical signatures were obtained by formulating and applying a five-stage modelling process that depicts the mining history of the area. The simulation results agree well with the concentrations and discharge trends measured in the mine drainage. Oxygen and meteoric water flow through the fractured continuum, leading to a high and steady release of hydrogen, iron, and sulfate ions derived from pyrite oxidation in the matrix continua closest to the fractures. Likewise, high chloride concentrations resulted from the mixing and gradual release of relatively immobile solutes in the matrix as they interacted with percolating water in the fracture. In both cases, the use of a multiple continua approach was essential to resolve sharp gradients for advection and faster kinetic reactions, while reducing the model’s dependence on block size for diffusive transport at the fracture–matrix interface. The model further allows for the calculation and analysis of solute exchange and transport in the unsaturated overburden resulting from rebound and imbibition processes, something pioneering when compared to other models in the field.
Originalsprache | Englisch |
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Seiten (von - bis) | 266-292 |
Seitenumfang | 27 |
Fachzeitschrift | Mine Water and the Environment |
Jahrgang | 42 |
Ausgabenummer | 2 |
DOIs | |
Publikationsstatus | Veröffentlicht - 15 Juni 2023 |
Bibliographische Notiz
Funding Information:The authors gratefully acknowledge the assistance of Professor Dr. Christoph von Hagke, Dr. Moritz Liebl, and Nicolas Villamizar M.Sc. from the Department of Environment & Biodiversity at the University of Salzburg for their advice with data management and manuscript construction. We also thank the team at RAG Anthrazit Ibbenbüren for facilitating discharge measurements and providing mine details. Our appreciation also goes to the Landesamt für Natur, Umwelt und Verbraucherschutz Nordrhein-Westfalen (LANUV) for supplying the study area’s precipitation data. Finally, we appreciate the comments and suggestions of the two anonymous reviewers and this journal’s editorial staff, who helped us to improve the manuscript’s quality.
Publisher Copyright:
© 2023, The Author(s).
Systematik der Wissenschaftszweige 2012
- 105 Geowissenschaften
Projekte
- 1 Abgeschlossen
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Reaktiver Stofftransport bei Flutung von stillgelegten Kohlebergwerken
Hilberg, S. (Projektleitung)
1/04/19 → 30/06/22
Projekt: Forschung